Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer

Liu Yu-Hang; Huang Ying; Xie Hua; Liu Cheng; Du Yuan-Yuan; Wang Rong; Li Jiang-Bo; Ji Yan-Ling

doi:doi:10.11648/j.rst.20230901.11

| Peer-Reviewed

Distribution Characteristics of ^⁷Be and ^²¹⁰Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O₃ Tracer

Liu Yu-Hang, Huang Ying, Xie Hua, Liu Cheng, Du Yuan-Yuan, Wang Rong, Li Jiang-Bo, Ji Yan-Ling

Published in Radiation Science and Technology (Volume 9, Issue 1)

Received: 2 January 2023 Accepted: 29 January 2023 Published: 27 February 2023

Views: Downloads:

Download PDF

Share This Article

Twitter
Linked In
Facebook

Abstract

In order to understand the quality of radiation environment in the near surface air in Mianyang area, to grasp the trend of its change, to explore the sources of aerosol substances near the surface and their significance in tracking the concentration of O₃ near the ground, a detailed gamma spectrum analysis of aerosol samples from March 2018 to February 2019 in Anzhou District, Jiangyou City, Zitong County and Pingwu County was carried out. In general, the activity concentration of ^⁷Be is higher in spring and autumn, while it is the lowest in summer. The annual average is 1.90-2.13mBq/m^³, which is basically the same as the distribution characteristics of inland, mid-latitude, and low-altitude areas in the world. The activity concentration of ^²¹⁰Pb is a "U" type distribution feature throughout the year. It is the lowest in late spring or early summer and has an annual average of 1.24-1.66mBq/m^³, which is a relatively high value of ^²¹⁰Pb activity concentration on global land. The correlation analysis between ^⁷Be and ^²¹⁰Pb and O₃ in near-surface aerosols showed that ^⁷Be and O₃ were weakly positively correlated, while the ratio of ^⁷Be/^²¹⁰Pb was significantly positively correlated with O₃, and ^²¹⁰Pb and O₃were significantly negatively correlated; The ^⁷Be/^²¹⁰Pb ratio can be used as a good tracer of O₃ sources in near-surface air. The O₃ source in the near surface air in Mianyang area is greatly affected by the vertical convection activity of the atmosphere.

Published in	Radiation Science and Technology (Volume 9, Issue 1)
DOI	10.11648/j.rst.20230901.11
Page(s)	1-7
Creative Commons	This is an Open Access article, distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium or format, provided the original work is properly cited.
Copyright	Copyright © The Author(s), 2023. Published by Science Publishing Group

Keywords

Aerosol, ^⁷Be, ^²¹⁰Pb, Distribution Characteristics, O₃, Tracing

References

[1]	M. Azahra, A. Camacho-Garcia. Seasonal 7Be concentrations in near-surface air of Granada (Spain) in the period 1993-2001, J. Appied Radiation and Isotopes, 59 (2003): 159-164.
[2]	H. L. ZHU, J. TANG, X. D. ZHENG. Applications of natural isotopes of 7Be and 210Pb in atmospheric science, J. Meteorological science and technology, 31 (2003): 131-135 (in Chinese).
[3]	F. B. ZHANG, M. Y. YANG, P. L. LIU, et al. A review on the behavior of 7Be in ecosystem, J. Journal of Nuclear Agricultural Science, 20 (2006): 444-448 (in Chinese).
[4]	H. W. Feely, R. J. Larsen, C. G. Sanderson. Factors that cause seasonal variations in beryllium-7 concentrations in surface air, J. J Environ Radioact, 9 (1989): 223-249.
[5]	J. R. Holton. Stratosphere/troposphere exchange & structure \| global aspects, J. Encyclopedia of Atmospheric Sciences, 2015, 257-261.
[6]	P. Zanis, E. Schuepbach, H. W. Giggeler, et al. Factors controlling beryllium-7 at Jungfraujoch in Switzerland, J. Tellus B, 51 (1999): 789-800.
[7]	UNSCEAR. Ionizing Radiation: Levels and EfectslM J, R. UNSCEAR 1972 Report, New York: UN, 1972.
[8]	C. Duefias, C. Femez, M. M. Perez. Radon-222 from the ocean Surface, J. Journal of Geophysical Research, 88 (1983): 8613.
[9]	J. Zhang, P. X. Li, Z. Li, et al. 210Pb and 210Po Activity Concentrations and Sources in Atmospheric Aerosol, J. Radiation Protection Bulletin, 6 (2015): 17-22 (in Chinese).
[10]	Compiled by Division of Monitoring Network, China Meteorological Administration. World Meteorological Organization: Global atmospheric monitoring phase 143, M. Beijing: Meteorological Publishing House, 2003 (in Chinese).
[11]	Z. Q. Pan. Monitoring and evaluation of ionizing radiation environment, M. Beijing: Atomic Energy Publishing House, 2007: 105-120 (in Chinese).
[12]	X. H. LI, Q. ZHAO, Q. WANG, et al. Application of 210Pb Analysis Method in Aerosol Determination of Chengdu, J. SICHUAN ENVIRONMENT, 36 (2017): 142-146 (in Chinese).
[13]	Z. G. BAI, G. J. WAN, C. S. WANG, et al. Distribution characteristics and erosion tracer of 7Be in the topsoil of Qinzhong Karst mountain area, J. Natural Science Progress, 7 (1997): 66-74.
[14]	Y. L. YANG, J. L. SHI, G. ZHANG, et al. Seasonal variations of beryllium-7 and typical POPs in aerosols from near-surface atmosphere in Guangzhou, China, J. GEOCHIMICA, 40 (2011): 72-82 (in Chinese).
[15]	G. J. WAN, X. D. ZHENG, H. N. LEE, et al. A comparative study on seasonal variation of 7Be concentrations in surface air between Mt. Waliguan and Mt. Guanfeng, J. GEOCHIMICA, 35 (2006): 221-226 (in Chinese).
[16]	Y. Z. CHANG, X. H. WANG, S. L. WANG, et al. Radionuclides monitoring in atmospheric aerosol samples in Xi’an, J. NUCLEAR TECHNIQUES, 31 (2008): 796-800 (in Chinese).
[17]	X. R. Jiang. 7Be content and its seasonal variation in the ground air around Hangzhou area, J. Nucl Sci Tech, 10 (1999): 230~234.
[18]	G. Q. LIU, Q. LUO, Y. H. PAN, et al. Variations of airborne 7Be in Shenzhen and its implication for atmospheric transport, J. GEOCHIMICA, 43 (2014): 32-38 (in Chinese).
[19]	D. M. Koch, D. J. Jacob, W. C. Graustein. Vertical transport of tropospheric aerosol as indicated by 7Be and 210Pb in a chemical tracer model, J. J Geophys Res, 101 (1996): 18651-18666.
[20]	H. E. Moore, S. E. Poet, E. A. Martell. 222Rn, 210Pb, 210Bi, and 210Po profiles and aerosol residence times versus altitude. Journal of Geophysics Research, 78 (1973): 7065-7075.
[21]	X. D. ZHENG, G. J. WAN, J. TANG, et al. Observation of 7Be and 210Pb in near-surface aerosols of Valiguan Mountains and their tracing of ozone concentration changes, J. Chinese science bulletin, 50 (2005): 72-76 (in Chinese).
[22]	A. Stohl, N. Spichtinger-Rakowsky, P. Bonasoni, et al. The influence of stratospheric intrusions on alpine ozone concentrations, J. Atmospheric Environment, 34 (2000): 1323-1354.
[23]	Liu, X., Fu, Y., Bi, Y., et al. Monitoring surface 10Be/7Be directly reveals stratospheric air intrusion in Sichuan Basin, China. Geophysical Research: Atmospheres, 127 (2022), e2022JD036543.
[24]	N. A. Wogman, C. W. Thomas, J. A. Cooper, et al. Cosmic Ray-Produced Radionuclides as Tracers of Atmospheric Precipitation Processes, J. Science, 159 (1968): 189-192.
[25]	W. Viezee and H. B. Singh. The distribution of beryllium-7 in the troposphere: implications on stratospheric/tropospheric air exchange, J. Geophysical research letters, 10 (1980): 805-808.

Cite This Article

Plain Text BibTeX RIS

APA Style

Liu Yu-Hang, Huang Ying, Xie Hua, Liu Cheng, Du Yuan-Yuan, et al. (2023). Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiation Science and Technology, 9(1), 1-7. https://doi.org/10.11648/j.rst.20230901.11

Copy | Download

ACS Style

Liu Yu-Hang; Huang Ying; Xie Hua; Liu Cheng; Du Yuan-Yuan, et al. Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiat. Sci. Technol. 2023, 9(1), 1-7. doi: 10.11648/j.rst.20230901.11

Copy | Download

AMA Style

Liu Yu-Hang, Huang Ying, Xie Hua, Liu Cheng, Du Yuan-Yuan, et al. Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiat Sci Technol. 2023;9(1):1-7. doi: 10.11648/j.rst.20230901.11

Copy | Download

@article{10.11648/j.rst.20230901.11,
  author = {Liu Yu-Hang and Huang Ying and Xie Hua and Liu Cheng and Du Yuan-Yuan and Wang Rong and Li Jiang-Bo and Ji Yan-Ling},
  title = {Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer},
  journal = {Radiation Science and Technology},
  volume = {9},
  number = {1},
  pages = {1-7},
  doi = {10.11648/j.rst.20230901.11},
  url = {https://doi.org/10.11648/j.rst.20230901.11},
  eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.rst.20230901.11},
  abstract = {In order to understand the quality of radiation environment in the near surface air in Mianyang area, to grasp the trend of its change, to explore the sources of aerosol substances near the surface and their significance in tracking the concentration of O3 near the ground, a detailed gamma spectrum analysis of aerosol samples from March 2018 to February 2019 in Anzhou District, Jiangyou City, Zitong County and Pingwu County was carried out. In general, the activity concentration of 7Be is higher in spring and autumn, while it is the lowest in summer. The annual average is 1.90-2.13mBq/m3, which is basically the same as the distribution characteristics of inland, mid-latitude, and low-altitude areas in the world. The activity concentration of 210Pb is a "U" type distribution feature throughout the year. It is the lowest in late spring or early summer and has an annual average of 1.24-1.66mBq/m3, which is a relatively high value of 210Pb activity concentration on global land. The correlation analysis between 7Be and 210Pb and O3 in near-surface aerosols showed that 7Be and O3 were weakly positively correlated, while the ratio of 7Be/210Pb was significantly positively correlated with O3, and 210Pb and O3 were significantly negatively correlated; The 7Be/210Pb ratio can be used as a good tracer of O3 sources in near-surface air. The O3 source in the near surface air in Mianyang area is greatly affected by the vertical convection activity of the atmosphere.},
 year = {2023}
}

Copy | Download

TY  - JOUR
T1  - Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer
AU  - Liu Yu-Hang
AU  - Huang Ying
AU  - Xie Hua
AU  - Liu Cheng
AU  - Du Yuan-Yuan
AU  - Wang Rong
AU  - Li Jiang-Bo
AU  - Ji Yan-Ling
Y1  - 2023/02/27
PY  - 2023
N1  - https://doi.org/10.11648/j.rst.20230901.11
DO  - 10.11648/j.rst.20230901.11
T2  - Radiation Science and Technology
JF  - Radiation Science and Technology
JO  - Radiation Science and Technology
SP  - 1
EP  - 7
PB  - Science Publishing Group
SN  - 2575-5943
UR  - https://doi.org/10.11648/j.rst.20230901.11
AB  - In order to understand the quality of radiation environment in the near surface air in Mianyang area, to grasp the trend of its change, to explore the sources of aerosol substances near the surface and their significance in tracking the concentration of O3 near the ground, a detailed gamma spectrum analysis of aerosol samples from March 2018 to February 2019 in Anzhou District, Jiangyou City, Zitong County and Pingwu County was carried out. In general, the activity concentration of 7Be is higher in spring and autumn, while it is the lowest in summer. The annual average is 1.90-2.13mBq/m3, which is basically the same as the distribution characteristics of inland, mid-latitude, and low-altitude areas in the world. The activity concentration of 210Pb is a "U" type distribution feature throughout the year. It is the lowest in late spring or early summer and has an annual average of 1.24-1.66mBq/m3, which is a relatively high value of 210Pb activity concentration on global land. The correlation analysis between 7Be and 210Pb and O3 in near-surface aerosols showed that 7Be and O3 were weakly positively correlated, while the ratio of 7Be/210Pb was significantly positively correlated with O3, and 210Pb and O3 were significantly negatively correlated; The 7Be/210Pb ratio can be used as a good tracer of O3 sources in near-surface air. The O3 source in the near surface air in Mianyang area is greatly affected by the vertical convection activity of the atmosphere.
VL  - 9
IS  - 1
ER  -

Copy | Download

Author Information

Liu Yu-Hang

Mianyang Radiation Environment Monitoring Station, Mian Yang, China
Huang Ying

Mianyang Radiation Environment Monitoring Station, Mian Yang, China
Xie Hua

Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mian Yang, China
Liu Cheng

Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mian Yang, China
Du Yuan-Yuan

Mianyang Radiation Environment Monitoring Station, Mian Yang, China
Wang Rong

Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mian Yang, China
Li Jiang-Bo

Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mian Yang, China
Ji Yan-Ling

Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mian Yang, China

Download PDF

Sections

Plain Text BibTeX RIS

APA Style

Liu Yu-Hang, Huang Ying, Xie Hua, Liu Cheng, Du Yuan-Yuan, et al. (2023). Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiation Science and Technology, 9(1), 1-7. https://doi.org/10.11648/j.rst.20230901.11

Copy | Download

ACS Style

Liu Yu-Hang; Huang Ying; Xie Hua; Liu Cheng; Du Yuan-Yuan, et al. Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiat. Sci. Technol. 2023, 9(1), 1-7. doi: 10.11648/j.rst.20230901.11

Copy | Download

AMA Style

Liu Yu-Hang, Huang Ying, Xie Hua, Liu Cheng, Du Yuan-Yuan, et al. Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer. Radiat Sci Technol. 2023;9(1):1-7. doi: 10.11648/j.rst.20230901.11

Copy | Download

@article{10.11648/j.rst.20230901.11,
  author = {Liu Yu-Hang and Huang Ying and Xie Hua and Liu Cheng and Du Yuan-Yuan and Wang Rong and Li Jiang-Bo and Ji Yan-Ling},
  title = {Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer},
  journal = {Radiation Science and Technology},
  volume = {9},
  number = {1},
  pages = {1-7},
  doi = {10.11648/j.rst.20230901.11},
  url = {https://doi.org/10.11648/j.rst.20230901.11},
  eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.rst.20230901.11},
  abstract = {In order to understand the quality of radiation environment in the near surface air in Mianyang area, to grasp the trend of its change, to explore the sources of aerosol substances near the surface and their significance in tracking the concentration of O3 near the ground, a detailed gamma spectrum analysis of aerosol samples from March 2018 to February 2019 in Anzhou District, Jiangyou City, Zitong County and Pingwu County was carried out. In general, the activity concentration of 7Be is higher in spring and autumn, while it is the lowest in summer. The annual average is 1.90-2.13mBq/m3, which is basically the same as the distribution characteristics of inland, mid-latitude, and low-altitude areas in the world. The activity concentration of 210Pb is a "U" type distribution feature throughout the year. It is the lowest in late spring or early summer and has an annual average of 1.24-1.66mBq/m3, which is a relatively high value of 210Pb activity concentration on global land. The correlation analysis between 7Be and 210Pb and O3 in near-surface aerosols showed that 7Be and O3 were weakly positively correlated, while the ratio of 7Be/210Pb was significantly positively correlated with O3, and 210Pb and O3 were significantly negatively correlated; The 7Be/210Pb ratio can be used as a good tracer of O3 sources in near-surface air. The O3 source in the near surface air in Mianyang area is greatly affected by the vertical convection activity of the atmosphere.},
 year = {2023}
}

Copy | Download

TY  - JOUR
T1  - Distribution Characteristics of 7Be and 210Pb in Near-Surface Aerosols in Mianyang Area and Their Significance to O3 Tracer
AU  - Liu Yu-Hang
AU  - Huang Ying
AU  - Xie Hua
AU  - Liu Cheng
AU  - Du Yuan-Yuan
AU  - Wang Rong
AU  - Li Jiang-Bo
AU  - Ji Yan-Ling
Y1  - 2023/02/27
PY  - 2023
N1  - https://doi.org/10.11648/j.rst.20230901.11
DO  - 10.11648/j.rst.20230901.11
T2  - Radiation Science and Technology
JF  - Radiation Science and Technology
JO  - Radiation Science and Technology
SP  - 1
EP  - 7
PB  - Science Publishing Group
SN  - 2575-5943
UR  - https://doi.org/10.11648/j.rst.20230901.11
AB  - In order to understand the quality of radiation environment in the near surface air in Mianyang area, to grasp the trend of its change, to explore the sources of aerosol substances near the surface and their significance in tracking the concentration of O3 near the ground, a detailed gamma spectrum analysis of aerosol samples from March 2018 to February 2019 in Anzhou District, Jiangyou City, Zitong County and Pingwu County was carried out. In general, the activity concentration of 7Be is higher in spring and autumn, while it is the lowest in summer. The annual average is 1.90-2.13mBq/m3, which is basically the same as the distribution characteristics of inland, mid-latitude, and low-altitude areas in the world. The activity concentration of 210Pb is a "U" type distribution feature throughout the year. It is the lowest in late spring or early summer and has an annual average of 1.24-1.66mBq/m3, which is a relatively high value of 210Pb activity concentration on global land. The correlation analysis between 7Be and 210Pb and O3 in near-surface aerosols showed that 7Be and O3 were weakly positively correlated, while the ratio of 7Be/210Pb was significantly positively correlated with O3, and 210Pb and O3 were significantly negatively correlated; The 7Be/210Pb ratio can be used as a good tracer of O3 sources in near-surface air. The O3 source in the near surface air in Mianyang area is greatly affected by the vertical convection activity of the atmosphere.
VL  - 9
IS  - 1
ER  -

Copy | Download